@article{Narun2021,

title = {Efficient Analysis of Photoluminescence Images for the Classification of Single-Photon Emitters},

author = {Leah R. Narun and Rebecca E. K. Fishman and Henry J. Shulevitz and Raj N. Patel and Lee C. Bassett},

url = {https://pubs.acs.org/doi/10.1021/acsphotonics.2c00795

https://arxiv.org/abs/2112.05654},

doi = {10.1021/acsphotonics.2c00795},

year  = {2022},

date = {2022-10-31},

journal = {ACS Photonics},

volume = {9},

number = {11},

pages = {3540–3549},

abstract = {Solid-state single-photon emitters (SPE) are a basis for emerging technologies such as quantum communication and quantum sensing. SPE based on fluorescent point defects are ubiquitous in semiconductors and insulators, and new systems with desirable properties for quantum information science may exist amongst the vast number of unexplored defects. However, the characterization of new SPE typically relies on time-consuming techniques for identifying point source emitters by eye in photoluminescence (PL) images. This manual strategy is a bottleneck for discovering new SPE, motivating a more efficient method for characterizing emitters in PL images. Here we present a quantitative method using image analysis and regression fitting to automatically identify Gaussian emitters in PL images and classify them according to their stability, shape, and intensity relative to the background. We demonstrate efficient emitter classification for SPEs in nanodiamond arrays and hexagonal boron nitride flakes. Adaptive criteria detect SPE in both samples despite variation in emitter intensity, stability, and background features. The detection criteria can be tuned for specific material systems and experimental setups to accommodate the diverse properties of SPE.},

keywords = {},

pubstate = {published},

tppubtype = {article}

}

@article{Shulevitz2021,

title = {Template-Assisted Self Assembly of Fluorescent Nanodiamonds for Scalable Quantum Technologies},

author = {Henry J. Shulevitz and Tzu-Yung Huang and Jun Xu and Steven Neuhaus and Raj N. Patel and Lee C. Bassett, Cherie R. Kagan},

url = {https://arxiv.org/abs/2111.14921},

doi = {10.1021/acsnano.1c09839},

year  = {2022},

date = {2022-01-13},

journal = {ACS Nano},

volume = {16},

number = {2},

pages = {1847–1856},

abstract = {Milled nanodiamonds containing nitrogen-vacancy (NV) centers provide an excellent platform for sensing applications as they are optically robust, have nanoscale quantum sensitivity, and form colloidal dispersions which enable bottom-up assembly techniques for device integration. However, variations in their size, shape, and surface chemistry limit the ability to position individual nanodiamonds and statistically study properties that affect their optical and quantum characteristics. Here, we present a scalable strategy to form ordered arrays of nanodiamonds using capillary-driven, template-assisted self assembly. This method enables the precise spatial arrangement of isolated nanodiamonds with diameters below 50 nm across millimeter-scale areas. Measurements of over 200 assembled nanodiamonds yield a statistical understanding of their structural, optical, and quantum properties. The NV centers' spin and charge properties are uncorrelated with nanodiamond size, but rather are consistent with heterogeneity in their nanoscale environment. This flexible assembly method, together with improved understanding of the material, will enable the integration of nanodiamonds into future quantum photonic and electronic devices.},

keywords = {},

pubstate = {published},

tppubtype = {article}

}

@article{Narun2021,

title = {Efficient Analysis of Photoluminescence Images for the Classification of Single-Photon Emitters},

author = {Leah R. Narun and Rebecca E. K. Fishman and Henry J. Shulevitz and Raj N. Patel and Lee C. Bassett},

url = {https://pubs.acs.org/doi/10.1021/acsphotonics.2c00795

https://arxiv.org/abs/2112.05654},

doi = {10.1021/acsphotonics.2c00795},

year  = {2022},

date = {2022-10-31},

journal = {ACS Photonics},

volume = {9},

number = {11},

pages = {3540–3549},

abstract = {Solid-state single-photon emitters (SPE) are a basis for emerging technologies such as quantum communication and quantum sensing. SPE based on fluorescent point defects are ubiquitous in semiconductors and insulators, and new systems with desirable properties for quantum information science may exist amongst the vast number of unexplored defects. However, the characterization of new SPE typically relies on time-consuming techniques for identifying point source emitters by eye in photoluminescence (PL) images. This manual strategy is a bottleneck for discovering new SPE, motivating a more efficient method for characterizing emitters in PL images. Here we present a quantitative method using image analysis and regression fitting to automatically identify Gaussian emitters in PL images and classify them according to their stability, shape, and intensity relative to the background. We demonstrate efficient emitter classification for SPEs in nanodiamond arrays and hexagonal boron nitride flakes. Adaptive criteria detect SPE in both samples despite variation in emitter intensity, stability, and background features. The detection criteria can be tuned for specific material systems and experimental setups to accommodate the diverse properties of SPE.},

keywords = {nanodiamond assembly, neurophysiology, nitrides, photon emission correlation spectroscopy, photon statistics},

pubstate = {published},

tppubtype = {article}

}

@article{Shulevitz2021,

title = {Template-Assisted Self Assembly of Fluorescent Nanodiamonds for Scalable Quantum Technologies},

author = {Henry J. Shulevitz and Tzu-Yung Huang and Jun Xu and Steven Neuhaus and Raj N. Patel and Lee C. Bassett, Cherie R. Kagan},

url = {https://arxiv.org/abs/2111.14921},

doi = {10.1021/acsnano.1c09839},

year  = {2022},

date = {2022-01-13},

journal = {ACS Nano},

volume = {16},

number = {2},

pages = {1847–1856},

abstract = {Milled nanodiamonds containing nitrogen-vacancy (NV) centers provide an excellent platform for sensing applications as they are optically robust, have nanoscale quantum sensitivity, and form colloidal dispersions which enable bottom-up assembly techniques for device integration. However, variations in their size, shape, and surface chemistry limit the ability to position individual nanodiamonds and statistically study properties that affect their optical and quantum characteristics. Here, we present a scalable strategy to form ordered arrays of nanodiamonds using capillary-driven, template-assisted self assembly. This method enables the precise spatial arrangement of isolated nanodiamonds with diameters below 50 nm across millimeter-scale areas. Measurements of over 200 assembled nanodiamonds yield a statistical understanding of their structural, optical, and quantum properties. The NV centers' spin and charge properties are uncorrelated with nanodiamond size, but rather are consistent with heterogeneity in their nanoscale environment. This flexible assembly method, together with improved understanding of the material, will enable the integration of nanodiamonds into future quantum photonic and electronic devices.},

keywords = {Condensed Matter, diamond NV center, nanodiamond assembly, Nanophotonics},

pubstate = {published},

tppubtype = {article}

}